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The objective of the present study is to observe whether there is a relationship between perceived social support, positive and negative affect and psychological well-being among married and widowed older adults. A non-probability purposive sampling technique was used to select a sample of 120 older adults, aged above 60 years, out of whom 60 were men (30 married and 30 widowed) and 60 women (30 married and 30 widowed). The Interpersonal Support Evaluation List (ISEL-12) (Cohen & Hoberman, 1983), Positive and Negative Affect Schedule (PANAS) (Watson, Clark, & Tellegen, 1988b) and Ryff’s Scales of Psychological Well-Being (Ryff, 1989) were administered to measure perceived social support, positive and negative affect and psychological well-being respectively. Significant differences were found between married and widowed older adults with respect to positive and negative affect and psychological well-being (p <0.05) There were no significant gender differences with respect to perceived social support, affect and psychological well-being. The study also showed significant correlations between the dimensions of perceived social support, positive and negative affect and psychological well-being (p<0.05). Details are discussed in the paper. The study brings to light that affect plays a significant role in the psychological well-being of older adults and encouraging of social networks can help sustain successful aging.